当前位置:网站首页>[2020] [paper notes] Based on Rydberg atom——
[2020] [paper notes] Based on Rydberg atom——
2022-07-23 18:45:00 【Su Nianxin】
Preface
type
Terahertz + The antenna Terahertz + The antenna Terahertz + The antenna
Periodical
Journal of Physics Journal of Physics Journal of Physics
author
Chen Zhiwen , Yu Zhenyue , Liao Kaiyu , Huang Wei , Yan Hui , Zhu Shiliang Chen Zhiwen , Yu Zhenyue , Liao Kaiyu , Huang Wei , Yan Hui , Zhu Shiliang Chen Zhiwen , Yu Zhenyue , Liao Kaiyu , Huang Wei , Yan Hui , Zhu Shiliang
Time
2020 2020 2020
Catalog
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Rydberg principle
Rydberg Atom means The main quantum number n > 10 n>10 n>10 Highly excited atom of
Rydberg The electric dipole moment of the atom is relatively low and the excited state is large 2 or 3 An order of magnitude
R y d b e r g Electric dipole moment ∝ n 2 Rydberg Electric dipole moment \propto n^2 Rydberg Electric dipole moment ∝n2
So for microwave 、THz The electric field of wave has extremely high sensitivity
( It can detect weak electric field signals )

Rydberg atom Strong coupling with electric field , bring Rydberg Electromagnetically induced transparency effect involving energy levels (EIT effect ) The transparent peak of AT split , The distance between the two peaks after splitting is proportional to the Rabi frequency of the coupling
Electromagnetically induced transparency effect (EIT effect ):
Be able to use Plus coherent light field To induce the atomic system Cancellation interference To counteract the absorption of certain light by the medium , Make opaque materials transparent
AT split :
Involving multiple electronic states and their interactions , It is a high-order nonlinear phenomenon of the interaction between intense laser and matter ?
Rabi frequency :
For a two-level system , We apply an electromagnetic wave , When the electromagnetic wave frequency is appropriate , The atoms in the system will continue E1 Energy levels and E2 Transition between energy levels , This phenomenon is called Rabi oscillation
Thus, the intensity measurement is transformed into frequency measurement by using quantum interference effect , Realize traceable and highly sensitive measurement of electromagnetic wave electric field intensity
Intensity measurement * Quantum interference effect frequency measurement Intensity measurement \overset{\text{ Quantum interference effect }}{\Longrightarrow} frequency measurement Intensity measurement * Quantum interference effect frequency measurement
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2012 Shaffer Group experiments
Coupling two through microwave field Rydberg The energy levels , utilize Rydberg Atomic EIT effect , And microwave AT split , Realize the precise measurement of microwave electric field intensity
sensitivity ≈ 30 μ V ⋅ c m − 1 ⋅ H z − 1 / 2 sensitivity \approx 30\mu V\cdot cm^{-1}\cdot Hz^{-1/2} sensitivity ≈30μV⋅cm−1⋅Hz−1/2
E m i n ≈ 8 μ V / c m E_{min}\approx 8\mu V/cm Emin≈8μV/cm
The probe light and the coupling light propagate in the opposite direction , In rubidium Rb In the atomic vapor chamber , Interact with atoms
- When there is no microwave , Observed Standard cascade three-level EIT Transparent peak
- When there is microwave field , Observed EIT Transparent peak , Split Into two peaks , spacing Δ f \Delta f Δf
Ω M W = 2 π Δ f \Omega _{MW}=2\pi \Delta f ΩMW=2πΔf
among Ω M W \Omega_{MW} ΩMW It's the Rabi frequency ( Coupled with microwave Rydberg Energy level )
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Considering scanning probe light , Doppler correction factor is introduced when detuning ?, Then the intensity of microwave electric field :
∣ E ∣ = ℏ μ Ω M W = 2 π ℏ μ λ p λ c Δ f |E|=\frac{\hbar}{ \mu }\Omega_{MW} = 2\pi \frac{\hbar}{\mu} \frac{\lambda _p}{ \lambda _c } \Delta f ∣E∣=μℏΩMW=2πμℏλcλpΔf
among μ \mu μ yes Rydberg Electric dipole moment of energy level , λ p \lambda_p λp Is the wavelength of detection light , λ c \lambda_c λc Is the wavelength of the coupling light
Convert the measurement of electric field strength into frequency measurement ( Because of all physical quantities , The frequency measurement accuracy is the highest )
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be based on Rydberg Atomic technology
1.THz Field strength measurement
Durham University Weatheril The team used three photons Rydberg state EIT, Measured 0.634THz Terahertz field strength

scanning Rydberg Laser Detuning , Record the probe light transmission
When detecting the detuning of light 、 When the detuning of the coupling light is zero , The four level Hamiltonian is :
H ^ 4 − l e v e l = ℏ 2 ( 0 Ω p 0 0 Ω p 2 Δ 1 p h Ω c 0 0 Ω c 2 Δ 2 p h Ω R 0 0 Ω R 2 ( Δ R + Δ 3 p h ) ) \hat{H}^{4-level} = \frac{\hbar}{2} \left( \begin{matrix} 0 & \Omega_p & 0 & 0 \\ \Omega_p & 2\Delta _{1ph} & \Omega_c & 0 \\ 0 & \Omega_c & 2\Delta_{2ph} & \Omega_R \\ 0 & 0 & \Omega_R& 2(\Delta _R + \Delta _{3ph} ) \end{matrix} \right) H^4−level=2ℏ⎝⎛0Ωp00Ωp2Δ1phΩc00Ωc2Δ2phΩR00ΩR2(ΔR+Δ3ph)⎠⎞
among
Δ 1 p h = v ⃗ ⋅ k ⃗ p \Delta _{1ph}=\vec{v} \cdot \vec{k}_p Δ1ph=v⋅kp
Δ 2 p h = v ⃗ ⋅ ( k ⃗ p + k ⃗ c ) \Delta _{2ph}=\vec{v} \cdot (\vec{k}_p+\vec{k}_c) Δ2ph=v⋅(kp+kc)
Δ 3 p h = v ⃗ ⋅ ( k ⃗ p + k ⃗ c + k ⃗ R ) \Delta _{3ph}=\vec{v} \cdot (\vec{k}_p+\vec{k}_c + \vec{k}_R ) Δ3ph=v⋅(kp+kc+kR)
v ⃗ \vec{v} v Is the atomic velocity
k p = 2 π / ( 852 n m ) {k}_p=2\pi/(852nm) kp=2π/(852nm) Is the number of detected light waves , Ω p \Omega_p Ωp It is the Rabi frequency of detection light
k c = 2 π / ( 1470 ) {k}_c=2\pi/(1470) kc=2π/(1470) Is the number of coupled light waves , Ω c \Omega_c Ωc Is the Rabi frequency of coupled light
k R = 2 π / ( 799 n m ) {k}_R=2\pi/(799nm) kR=2π/(799nm) yes Rydberg Number of light waves , Ω R \Omega_R ΩR yes Rydberg Optical Rabi frequency
Δ R \Delta _R ΔR yes Rydberg Light detuning
For further study EIT-AT split , introduce 0.634THz Field coupling 21 P 3 / 2 → 21 S 1 / 2 21P_{3/2}\rightarrow 21 S_{1/2} 21P3/2→21S1/2 bring EIT The window splits into two peaks
⋮ \vdots ⋮
⋮ \vdots ⋮
After opening the terahertz field , Use double Lorentz linetype to fit data
Limit for each Lorenz peak Width , To match EIT Cleavage peak ,
The height of the peak 、 The bimodal spacing is set as a free parameter , Fit the curve
extract EIT The cleavage peak corresponds to THz Rabi frequency Ω T / 2 π = ( 5.2 ± 1.4 ) M H z \Omega_T/2\pi = (5.2 \pm 1.4) MHz ΩT/2π=(5.2±1.4)MHz,
It can be calculated that THz Field strength ( 25 ± 5 ) m V ⋅ c m − 1 (25\pm 5)mV\cdot cm^{-1} (25±5)mV⋅cm−1
specific Rydberg States can only be coupled to a few terahertz frequencies close to resonance , But you can choose different Rydberg States to couple different frequencies , Realize the detection of wide terahertz frequency domain .
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2.THz Near field high-speed imaging
Convert the hard to detect terahertz signal into other easy to detect signals , For example, electrical signals
- In the early : With spatial distribution THz Ionization Rydberg atom , The generated ions are focused on a spatially resolved microchannel plate , Realize to THz Spatially distinguishable detection of field strength ( shortcoming : Yes Rydberg Atoms are destructive , Disposable , Low resolution )
- 2016: use THz Pumping Rydberg atom , Through spontaneous emission , The fluorescence in the visible light band , Imaging —— Realized THz Near field real-time imaging of spatial distribution of field strength

Infrared laser beam and THz Beam coaxial alignment , Through the 2 mm Long quartz saturated bubbles
At the spatial overlapping position of terahertz field and laser beam, the atom is excited to 21 S 1 / 2 21S_{1/2} 21S1/2 Of Rydberg state , And emit fluorescence in the visible light band
The laser beam and terahertz wave pass horizontally through the imaging area , Some terahertz waves are reflected to produce standing wave interference structures
This imaging technology does not require repeated data acquisition or scanning
Detector location , So imaging is real-time . The bandwidth limit of imaging is determined by Rydberg Energy level lifetime determines , Generally about Microsecond Magnitude
⋮ \vdots ⋮
⋮ \vdots ⋮
Using high-speed rotating optical chopper ( Rotating blade with adjustable frequency ), It can verify the high-speed performance of the imaging system
- Reduce the thickness of cesium bubble chamber + Enhance anti reflection layer , Sure Improve image quality
- The more advanced THz lens, Sure Improve image resolution
- Enlarge the cesium bubble chamber to expand THz Area of Sensor , Form a larger atomic excitation surface , Increase the imaging area
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3.THz signal communication
- Compared with microwave communication , Large bandwidth 、 Large capacity
- Compared with laser communication , For platform stability 、 Low requirements for follow-up
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The picture below is Rydberg Atomic digital communication experimental device and energy level system
Connect baseband digital signal with Rydberg Microwave mixing of atomic resonance ( The sender )
Microwave signal absorption mixing occurs EIT-AT split , Will receive Band signal Converted to probe light Amplitude phase φ μ \varphi_\mu φμ
External use heterodyne probe , Phase demodulation is carried out through the lock-in amplifier
φ μ = a r c t a n ( V Q / V I ) \varphi_\mu=arctan(V_Q/V_I) φμ=arctan(VQ/VI)
take Phase information Turn into Quadrature phase change voltage signal

(f) The demodulated co directional voltage signal is given V I V_I VI Examples with five different coding phases
(g)(h) It is the phase signal and phase trajectory of the signal receiving end (8PSK)
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Rydberg atom Antenna
The following is based on a four level atomic system THz Communication scheme

6 S 1 / 2 ( F = 4 ) 6S_{1/2}(F=4) 6S1/2(F=4) Of Cs The atom is in ∣ 1 * |1\rangle ∣1*
6 P 3 / 2 ( F ′ = 5 ) 6P_{3/2}(F'=5) 6P3/2(F′=5) Of Cs The atom is in ∣ 2 * |2\rangle ∣2*
25 S 1 / 2 ( F ′ = 5 ) 25S_{1/2}(F'=5) 25S1/2(F′=5) Of Cs The atom is in ∣ 3 * |3\rangle ∣3*
25 P 3 / 2 ( F ′ = 5 ) 25P_{3/2}(F'=5) 25P3/2(F′=5) Of Cs The atom is in ∣ 4 * |4\rangle ∣4*
- Detection light wavelength 852 n m 852nm 852nm, coupling ∣ 1 * ∣ 2 * |1\rangle\leftrightarrow |2\rangle ∣1*∣2* Ecological transition , Corresponding to Rabi frequency Ω p \Omega_p Ωp
- Coupling light wavelength 515 n m 515nm 515nm, coupling ∣ 2 * ∣ 3 * |2\rangle\leftrightarrow |3\rangle ∣2*∣3* Ecological transition , Corresponding to Rabi frequency Ω c \Omega_c Ωc
- Use 338.75 G H z 338.75GHz 338.75GHz Of THz site , For coupling two Rydberg state ∣ 3 * ∣ 4 * |3\rangle\leftrightarrow |4\rangle ∣3*∣4* Ecological transition , The corresponding Rabi frequency is Ω T \Omega_T ΩT
Four level Hamiltonian H 4 − l e v e l H^{4-level} H4−level Expressed as
H = ℏ { Ω p ∣ 1 * * 2 ∣ + Ω c ∣ 2 * * 3 ∣ + Ω T ∣ 3 * * 4 ∣ − Δ p ∣ 2 * * 2 ∣ − ( Δ p + Δ c ) ∣ 3 * * 3 ∣ − ( Δ p + Δ c − Δ T ) ∣ 4 * * 4 ∣ + h . c . } H = \hbar \{ \Omega_p|1\rangle\langle2| + \Omega_c|2\rangle\langle3| +\Omega_T|3\rangle\langle4| - \\\Delta _p|2\rangle\langle2| - (\Delta _p+\Delta_c)|3\rangle\langle3| - \\ (\Delta _p+\Delta_c - \Delta _T) |4\rangle\langle4| + h.c. \} H=ℏ{ Ωp∣1**2∣+Ωc∣2**3∣+ΩT∣3**4∣−Δp∣2**2∣−(Δp+Δc)∣3**3∣−(Δp+Δc−ΔT)∣4**4∣+h.c.}
among
Rabi frequency
Ω p = μ 12 E p / ℏ \Omega_p=\mu_{12}E_p/\hbar Ωp=μ12Ep/ℏ
Ω c = μ 23 E c / ℏ \Omega_c=\mu_{23}E_c/\hbar Ωc=μ23Ec/ℏ
Ω T = μ 34 E T / ℏ \Omega_T=\mu_{34}E_T/\hbar ΩT=μ34ET/ℏ
Detuning
Δ p = ω p − ω 12 \Delta_p = \omega_p - \omega_{12} Δp=ωp−ω12
Δ c = ω c − ω 23 \Delta_c = \omega_c - \omega_{23} Δc=ωc−ω23
Δ T = ω T − ω 34 \Delta_T = \omega_T - \omega_{34} ΔT=ωT−ω34
The detection light is a weak field , When Ω c = 2 π × 5.72 M H z \Omega_c=2\pi\times 5.72MHz Ωc=2π×5.72MHz,THz Rabi frequency Ω T = 2 π × [ 0 , 1 , 2.5 , 5 ] M H z \Omega_T=2\pi \times [ 0,1,2.5,5 ] MHz ΩT=2π×[0,1,2.5,5]MHz when ,EIT-AT The split result is shown in the right figure (b)
Yes THz The carrier is amplitude modulated AM, Got EIT The signal will also have modulation information
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Purpose + Conclusion
Rydberg Atoms have great electric dipole moments in the microwave and terahertz bands , Using the quantum interference effect, the electromagnetic wave field strength of this frequency band can be Highly sensitive detection , Theoretically, the sensitivity can be much higher than that of the existing detection technology
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problem
Rydberg What structure is used for atomic antenna ?
On the left vector of Quantum States 、 How is the right vector calculated ?
The function and significance of Hamiltonian ?
Is the sum of the kinetic energy of all particles plus the potential energy of the particles related to the system
For different cases or numbers of particles , Hamiltonian is different
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